Han, H., Kim, K. M., Lee, C. W., Lee, C. S., Pawar, R. C., Jones, J. L., Hong, Y. R., Ryu, J. H., Song, T., Kang, S. H., Choi, H., & Mhin, S. (2017). Few-layered metallic 1T-MoS2/TiO2 with exposed (001) facets: Two-dimensional nanocomposites for enhanced photocatalytic activities. Physical Chemistry Chemical Physics, 19(41), 28207-28215. https://doi.org/10.1039/c7cp05523d
Han, Hyuksu ; Kim, Kang Min ; Lee, Chan Woo et al. / Few-layered metallic 1T-MoS2/TiO2 with exposed (001) facets : Two-dimensional nanocomposites for enhanced photocatalytic activities. In: Physical Chemistry Chemical Physics. 2017 ; Vol. 19, No. 41. pp. 28207-28215.
@article{8eae4fe074384970be092cec1a28fad8,
title = "Few-layered metallic 1T-MoS2/TiO2 with exposed (001) facets: Two-dimensional nanocomposites for enhanced photocatalytic activities",
abstract = "Titanium dioxide (TiO2) with exposed (001) facets (TiO2(001)) has attractive photocatalytic properties. However, the high recombination rate of the photo-excited charge carriers on this surface often limits its application. Here, we report that a few-layered 1T-MoS2 coating on TiO2(001) nanosheets (abbreviated as MST) can be a promising candidate that overcomes some of the challenges of TiO2(001). Computational and experimental results demonstrate that MST as a photocatalyst exhibits a significantly low-charge recombination rate as well as excellent long-term durability. The synthesized MST 2D nanocomposites show a 31.9% increase in photocatalytic activity for hydrogen (H2) production relative to the counterpart TiO2(001). MST offers a new route for further improvement of the photocatalytic activity of TiO2 with exposed high energy facets.",
author = "Hyuksu Han and Kim, {Kang Min} and Lee, {Chan Woo} and Lee, {Caroline S.} and Pawar, {Rajendra C.} and Jones, {Jacob L.} and Hong, {Yu Rim} and Ryu, {Jeong Ho} and Taeseup Song and Kang, {Suk Hyun} and Heechae Choi and Sungwook Mhin",
note = "Publisher Copyright: {\textcopyright} the Owner Societies 2017.",
year = "2017",
doi = "10.1039/c7cp05523d",
language = "English",
volume = "19",
pages = "28207--28215",
journal = "Physical Chemistry Chemical Physics",
issn = "1463-9076",
number = "41",
}
Han, H, Kim, KM, Lee, CW, Lee, CS, Pawar, RC, Jones, JL, Hong, YR, Ryu, JH, Song, T, Kang, SH, Choi, H & Mhin, S 2017, 'Few-layered metallic 1T-MoS2/TiO2 with exposed (001) facets: Two-dimensional nanocomposites for enhanced photocatalytic activities', Physical Chemistry Chemical Physics, vol. 19, no. 41, pp. 28207-28215. https://doi.org/10.1039/c7cp05523d
Few-layered metallic 1T-MoS2/TiO2 with exposed (001) facets: Two-dimensional nanocomposites for enhanced photocatalytic activities. / Han, Hyuksu; Kim, Kang Min; Lee, Chan Woo et al.
In:
Physical Chemistry Chemical Physics, Vol. 19, No. 41, 2017, p. 28207-28215.
Research output: Contribution to journal › Article › peer-review
TY - JOUR
T1 - Few-layered metallic 1T-MoS2/TiO2 with exposed (001) facets
T2 - Two-dimensional nanocomposites for enhanced photocatalytic activities
AU - Han, Hyuksu
AU - Kim, Kang Min
AU - Lee, Chan Woo
AU - Lee, Caroline S.
AU - Pawar, Rajendra C.
AU - Jones, Jacob L.
AU - Hong, Yu Rim
AU - Ryu, Jeong Ho
AU - Song, Taeseup
AU - Kang, Suk Hyun
AU - Choi, Heechae
AU - Mhin, Sungwook
N1 - Publisher Copyright:
© the Owner Societies 2017.
PY - 2017
Y1 - 2017
N2 - Titanium dioxide (TiO2) with exposed (001) facets (TiO2(001)) has attractive photocatalytic properties. However, the high recombination rate of the photo-excited charge carriers on this surface often limits its application. Here, we report that a few-layered 1T-MoS2 coating on TiO2(001) nanosheets (abbreviated as MST) can be a promising candidate that overcomes some of the challenges of TiO2(001). Computational and experimental results demonstrate that MST as a photocatalyst exhibits a significantly low-charge recombination rate as well as excellent long-term durability. The synthesized MST 2D nanocomposites show a 31.9% increase in photocatalytic activity for hydrogen (H2) production relative to the counterpart TiO2(001). MST offers a new route for further improvement of the photocatalytic activity of TiO2 with exposed high energy facets.
AB - Titanium dioxide (TiO2) with exposed (001) facets (TiO2(001)) has attractive photocatalytic properties. However, the high recombination rate of the photo-excited charge carriers on this surface often limits its application. Here, we report that a few-layered 1T-MoS2 coating on TiO2(001) nanosheets (abbreviated as MST) can be a promising candidate that overcomes some of the challenges of TiO2(001). Computational and experimental results demonstrate that MST as a photocatalyst exhibits a significantly low-charge recombination rate as well as excellent long-term durability. The synthesized MST 2D nanocomposites show a 31.9% increase in photocatalytic activity for hydrogen (H2) production relative to the counterpart TiO2(001). MST offers a new route for further improvement of the photocatalytic activity of TiO2 with exposed high energy facets.
UR - http://www.scopus.com/inward/record.url?scp=85032641318&partnerID=8YFLogxK
U2 - 10.1039/c7cp05523d
DO - 10.1039/c7cp05523d
M3 - Article
C2 - 29026899
AN - SCOPUS:85032641318
SN - 1463-9076
VL - 19
SP - 28207
EP - 28215
JO - Physical Chemistry Chemical Physics
JF - Physical Chemistry Chemical Physics
IS - 41
ER -
Han H, Kim KM, Lee CW, Lee CS, Pawar RC, Jones JL et al. Few-layered metallic 1T-MoS2/TiO2 with exposed (001) facets: Two-dimensional nanocomposites for enhanced photocatalytic activities. Physical Chemistry Chemical Physics. 2017;19(41):28207-28215. doi: 10.1039/c7cp05523d
